Experimental screening and selection criteria of natural coagulants towards wastewater treatment
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Abstract
The search for eco-friendly materials has greatly evolved ahead of basic requirements encompassing sustainable practices. The selection of such sustainable material requires procedural systematic screening tests to facilitate decision-making. Water and wastewater treatment processes involve several chemicals, and they need to transition from commercial to natural materials owing to their environmental and economic concerns. The present study aimed to select and screen natural coagulants for wastewater treatment. The criteria assessment factors for the present study were easy availability, economic value, turbidity removal efficiency, and reduced sludge generation with high dewaterability. A standard jar test apparatus was used for the coagulation experimental runs. The physicochemical parameters were analyzed using standard methods. The results presented positive insights into the efficiency of tested natural coagulants, with the least turbidity removal of 83.3% by rice husk at 1gm/500ml and the highest being 96.4% by onion peel at 1gm/500ml. The sludge obtained after treatment with natural coagulants has presented an excellent dewaterability, with the least being 29.17% by tamarind seeds at 1gm/500ml and the maximum being 90.2% by coconut fibre at 1gm/500ml. From the study, was concluded that the screening method promoted the selection of the best coagulant type and dose and reduced the efforts and time needed to eliminate the non-performers.
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Coagulation, Natural coagulants, Screening, Sludge, Turbidity, Wastewater
Abood, M. M., Azhari, N. N. B. & Abdelmoneim, A. O. (2017). The use of peanut and sesame seeds as natural coagulant in the water treatment. Infrastructure University Kuala Lumpur Research Journal, 5(1), 1-10.
Ahmad, A., Kurniawan, S. B., Abdullah, S. R. S., Othman, A. R. & Hasan, H. A. (2022). Exploring the extraction methods for plant-based coagulants and their future approaches. Science of the Total Environment, 818, 151668. https://doi.org/10.1016/j.scitotenv.2021.151668
Ahmed, S. N., Bhargava, M. & KV, S. S. (2023). Material selection using knowledge-based expert system for racing bicycle forks. Intelligent Systems with Applications, 19, 200257. https://doi.org/10.1016/j.iswa.2023.200257
Alam Bhuiyan, M. M. & Hammad, A. (2023). A hybrid multi-criteria decision support system for selecting the most sustainable structural material for a multistory building construction. Sustainability, 15(4), 3128. https://doi.org/10.3390/su15043128
Al-Jadabi, N., Laaouan, M., El Hajjaji, S., Mabrouki, J., Benbouzid, M. & Dhiba, D. (2023). The dual performance of Moringa oleifera seeds as eco-friendly natural coagulant and as an antimicrobial for wastewater treatment: a review. Sustainability, 15(5), 4280. https://doi.org/10.3390/su15054280
APHA (2017). Standard Methods for the Examination of Water and Wastewater (23rd ed.). Washington DC: American Public Health Association.
Ashby, M. F. (1994). Materials selection in mechanical design. Metallurgia Italiana, 86, 475-475.
Badawi, A. K. & Zaher, K. (2021). Hybrid treatment system for real textile wastewater remediation based on coagulation/flocculation, adsorption and filtration processes: performance and economic evaluation. Journal of Water Process Engineering, 40, 101963. https://doi.org/10.1016/j.jwpe.2021.101963
Benalia, A., Baatache, O., Derbal, K., Khalfaoui, A., Amrouci, Z., Pizzi, A. & Panico, A. (2024). The use of central composite design (CCD) to optimize and model the coagulation-flocculation process using a natural coagulant: Application in jar test and semi-industrial scale. Journal of Water Process Engineering, 57, 104704. https://doi.org/10.1016/j.jwpe.2023.104704
Cai, L., Sun, J., Cui, L., Jiang, Y. & Huang, Z. (2020). Stabilization of heavy metals in piggery wastewater sludge through coagulation-hydrothermal reaction–pyrolysis process and sludge biochar for tylosin removal. Journal of cleaner production, 260, 121165. https://doi.org/10.1016/j.jclepro.2020.121165
Charcosset, C. (2022). Classical and recent developments of membrane processes for desalination and natural water treatment. Membranes, 12(3), 267. https://doi.org/10.3390/membranes12030267
Craven, D., Eisenhauer, N., Pearse, W. D., Hautier, Y., Isbell, F., Roscher, C. & Manning, P. (2018). Multiple facets of biodiversity drive the diversity–stability relationship. Nature Ecology & Evolution, 2(10), 1579-1587. https://doi.org/10.1038/s41559-018-0647-7
Dayarathne, H. N. P., Angove, M. J., Aryal, R., Abuel-Naga, H., & Mainali, B. (2021). Removal of natural organic matter from source water: Review on coagulants, dual coagulation, alternative coagulants, and mechanisms. Journal of Water Process Engineering, 40, 101820. https://doi.org/10.1016/j.jwpe.2020.101820
Deng, X., & Yu, Z. (2022). A systematic review of machine-translation-assisted language learning for sustainable education. Sustainability, 14(13), 7598. https://doi.org/10.3390/su14137598
Diver, D., Nhapi, I. & Ruziwa, W. R. (2023). The potential and constraints of replacing conventional chemical coagulants with natural plant extracts in water and wastewater treatment. Environmental Advances, 100421. https://doi.org/10.1016/j.envadv.2023.100421
Duggireddy, R. P. & Pisharody, L. (2024). Traditional methods of water purification in rural areas. In Water Resources Management for Rural Development (pp. 55-64). Elsevier. https://doi.org/10.1016/B978-0-443-18778-0.00003-9
El-taweel, R. M., Mohamed, N., Alrefaey, K. A., Husien, S., Abdel-Aziz, A. B., Salim, A. I., ... & Radwan, A. G. (2023). A review of coagulation explaining its definition, mechanism, coagulant types, and optimization models; RSM, and ANN. Current Research in Green and Sustainable Chemistry, 6, 100358. https://doi.org/10.1016/j.crgsc.2023.100358
Febrianti, N., Permana, R. N. W. & Ariani, I. K. (2024). Utilization of aloe vera as a biocoagulant for turbidity, total dissolved solid (TDS), and iron (Fe) removal in well water. In IOP Conference Series: Earth and Environmental Science (Vol. 1312, No. 1, p. 012007). IOP Publishing. 10.1088/1755-1315/1312/1/012007
Findik, F. & Turan, K. (2012). Materials selection for lighter wagon design with a weighted property index method. Materials & Design, 37, 470-477. https://doi.org/10.1016/j.matdes.2012.01.016
Gutub, S. A., Bassyouni, M. & Abdel-Hamid, S. M. S. (2013). Dissolved solids adsorption of freshwater using synthesized bio-foam composite. Life Science Journal, 10(2), 464-471.
Hadadi, A., Imessaoudene, A., Bollinger, J. C., Bouzaza, A., Amrane, A., Tahraoui, H. & Mouni, L. (2023). Aleppo pine seeds (Pinus halepensis Mill.) as a promising novel green coagulant for the removal of Congo red dye: Optimization via machine learning algorithm. Journal of Environmental Management, 331, 117286. https://doi.org/10.1016/j.jenvman.2023.117286
Hu, P., Ren, J., Ren, W., Sun, Y. & Yang, H. (2024). The feasibility and mechanism of poly-aluminum/titanium silicate composite coagulants for the efficient removal of nano-and micro-sized plastics. Chemical Engineering Journal, 482, 149095. https://doi.org/10.1016/j.cej.2024.149095
Jagaba, A. H., Birniwa, A. H., Usman, A. K., Mu'azu, N. D., Yaro, N. S. A., Soja, U. B., ... & Lawal, I. M. (2023). Trend and current practices of coagulation-based hybrid systems for pulp and paper mill effluent treatment: mechanisms, optimization techniques and performance evaluation. Journal of Cleaner Production, 139543. https://doi.org/10.1016/j.jclepro.2023.139543
Jasim, N. A., Azeez, J. M. & Shamkhi, M. S. (2022). A comparative study of different coagulants used in treatment of turbid water. Open Engineering, 12(1), 890-904. https://doi.org/10.1515/eng-2022-0366
Joaquin, A. A., Sivamani, S. & Gnanasundaram, N. (2024). Statistical experimental design and analysis of mixed natural-synthetic coagulants for the reduction of total suspended solids and turbidity in sewage wastewater treatment. Biomass Conversion and Biorefinery, 14(4), 4583-4590. https://doi.org/10.1007/s13399-022-02566-2
Karnena, M. K. & Saritha, V. (2022). Phytochemical and physicochemical screening of plant-based materials as coagulants for turbidity removal–An unprecedented approach. Watershed Ecology and the Environment, 4, 188-201. https://doi.org/10.1016/j.wsee.2022.11.006
Kingue, B., Njila, R. & Ndongo, B. (2023). Assessment of groundnut (Arachis hypogaea) as a natural coagulant for water treatment. Water Practice & Technology, 18(9), 2057-2067.
Knap-Bałdyga, A. & Żubrowska-Sudoł, M. (2023). Natural Organic Matter Removal in Surface Water Treatment via Coagulation—Current Issues, Potential Solutions, and New Findings. Sustainability, 15(18), 13853. https://doi.org/10.2166/wpt.2023.127
Koul, B., Bhat, N., Abubakar, M., Mishra, M., Arukha, A. P. & Yadav, D. (2022). Application of natural coagulants in water treatment: A sustainable alternative to chemicals. Water, 14(22), 3751. https://doi.org/10.3390/w14223751
Kumar, S. & Singh, R. (2007). A short note on an intelligent system for selection of materials for progressive die components. Journal of Materials Processing Technology, 182(1-3), 456-461. https://doi.org/10.1016/j.jmatprotec.2006.09.004
Li, H., Li, Z., Wang, P., Liu, Z., An, L., Zhang, X., ... & Gao, W. (2024). Evaluation of citrus pectin extraction methods: Synergistic enhancement of pectin's antioxidant capacity and gel properties through combined use of organic acids, ultrasonication, and microwaves. International Journal of Biological Macromolecules, 266, 131164. https://doi.org/10.1016/j.ijbiomac.2024.131164
Louhichi, G., El Khouni, A., Ghrabi, A. & Khouni, I. (2024). Phytotoxicity assessment of treated vegetable oily wastewater via environmentally coagulation/flocculation and membrane filtration technologies using lettuce (Lactuca sativa) seeds. Environmental Science and Pollution Research, 1-25. https://doi.org/10.1007/s11356-023-31594-2
Merayo, D., Rodriguez-Prieto, A. & Camacho, A. M. (2019). Comparative analysis of artificial intelligence techniques for material selection applied to manufacturing in Industry 4.0. Procedia Manufacturing, 41, 42-49. https://doi.org/10.1016/j.promfg.2019.07.027
Mohd-Asharuddin, S., Othman, N., Zin, N. S. M. & Tajarudin, H. A. (2017). A chemical and morphological study of cassava peel: A potential waste as coagulant aid. In MATEC web of conferences (Vol. 103, p. 06012). EDP Sciences. https://doi.org/10.1051/matecconf/201710306012
Mohd-Salleh, S. N. A., Shaylinda, M. Z. N., Othman, N., Yasni, G. & Norshila, A. B. (2020). Optimization of tapioca peel powder as natural coagulant in removing chemical oxygen demand, ammonia nitrogen, turbidity, colour, and suspended solids from leachate sample. Water and Environmental Engineering, 69-86.
Mujariah, M., Abram, P. H. & Jura, M. R. (2017). Penggunaan Gel Lidah Buaya (Aloe Vera) Sebagai Koagulan Alami Dalam Penjernihan Air Sumur Di Desa Sausu Tambu Kecamatan Sausu. Jurnal Akademika Kimia, 5(1), 16-22.
Muniraj, S., Muthunarayanan, V., Venkataraman, S., Sunitha, T. G. & Thamaraiselvi, C. (2023). Drinking water treatment with natural coagulants—a promising alternative for sustainable water usage. Resource Recovery in Drinking Water Treatment, 107-127. https://doi.org/10.1016/B978-0-323-99344-9.00008-6
Nellippallil, A. B., Allen, J. K., Gautham, B. P., Singh, A. K., Mistree, F., Nellippallil, A. B., ... & Mistree, F. (2020). Integrated design of materials, products, and associated manufacturing processes. Architecting Robust Co-Design of Materials, Products, and Manufacturing Processes, 1-45. https://doi.org/10.1007/978-3-030-45324-4_1
Nguyet, P. N., Hata, Y., Maharjan, N., Watari, T., Hatamoto, M. & Yamaguchi, T. (2020). Adsorption of colour from dye wastewater effluent of a down-flow hanging sponge reactor on purified coconut fibre. Environmental technology, 41(10), 1337-1346. · https://doi.org/10.1080/09593330.2018.1534000
Ntwampe, I. O. (2021). Treatment of AMD using a combination of saw dust, bentonite clay and phosphate in the removal of turbid materials and toxic metals. Water Practice & Technology, 16(2), 541-556. https://doi.org/10.2166/wpt.2021.014
Ogunshina, M. S., Abioye, O. M., Adeniran, K. A. & Olasehinde, D. A. (2023). Moringa Oleifera Coagulation Characteristics in Wastewater Treatment in a University Dormitory. Nature Environment and Pollution Technology, 22(2), 699-707. https://doi.org/10.46488/NEPT.2023.v22i02.013
Owodunni, A. A. & Ismail, S. (2021). Revolutionary technique for sustainable plant-based green coagulants in industrial wastewater treatment—A review. Journal of Water Process Engineering, 42, 102096. https://doi.org/10.1016/j.jwpe.2021.102096
Putra, R. S., Amri, R. Y. & Ayu, M. (2020). Turbidity removal of synthetic wastewater using biocoagulants based on protein and tannin. In AIP conference proceedings (Vol. 2242, No. 1). AIP Publishing. https://doi.org/10.1063/5.0007846
Ragio, R. A., Arantes, C. C., García, J. & Subtil, E. L. (2023). Assessment of natural tannin-based coagulant for effective ultrafiltration (UF) of UASB effluent: Fouling mechanisms, pollutant removal and water reclamation feasibility. Journal of Environmental Chemical Engineering, 11(3), 109778. https://doi.org/10.1016/j.jece.2023.109778
Ramutshatsha-Makhwedzha, D., Mavhungu, A., Moropeng, M. L. & Mbaya, R. (2022). Activated carbon derived from waste orange and lemon peels for the adsorption of methyl orange and methylene blue dyes from wastewater. Heliyon, 8(8). https://doi.org/10.1016/j.heliyon.2022.e09930
Sahu, A., Dosi, R., Kwiatkowski, C., Schmal, S. & Poler, J. C. (2023). Advanced polymeric nanocomposite membranes for water and wastewater treatment: a comprehensive review. Polymers, 15(3), 540. https://doi.org/10.3390/polym15030540
Said, N. S. M., Abdullah, S. R. S., Ismail, N. I., Hasan, H. A. & Othman, A. R. (2023). Integrating treatment processes of coffee processing mill effluent for reclamation of secondary resources. Journal of Cleaner Production, 386, 135837. https://doi.org/10.1016/j.jclepro.2022.135837
Saleem, M., & Bachmann, R. T. (2019). A contemporary review on plant-based coagulants for applications in water treatment. Journal of Industrial and Engineering Chemistry, 72, 281-297. https://doi.org/10.1016/j.jiec.2018.12.029
Saleh, T. A., Mustaqeem, M. & Khaled, M. (2022). Water treatment technologies in removing heavy metal ions from wastewater: A review. Environmental Nanotechnology, Monitoring & Management, 17, 100617. https://doi.org/10.1016/j.enmm.2021.100617
Sapuan, S. M. & Abdalla, H. S. (1998). A prototype knowledge-based system for the material selection of polymeric-based composites for automotive components. Composites Part A: Applied Science and Manufacturing, 29(7), 731-742. https://doi.org/10.1016/S1359-835X(98)00049-9
Saritha, V., Karnena, M. K. & Dwarapureddi, B. K. (2019). “Exploring natural coagulants as impending alternatives towards sustainable water clarification”–a comparative studies of natural coagulants with alum. Journal of Water Process Engineering, 32, 100982. https://doi.org/10.1016/j.jwpe.2019.100982
Shaharuzaman, M. A., Sapuan, S. M., & Mansor, M. R. (2021). Sustainable materials selection: principles and applications. In Design for Sustainability (pp. 57-84). Elsevier. https://doi.org/10.1016/B978-0-12-819482-9.00001-0
Sharma, V., Zivic, F., Adamovic, D., Ljusic, P., Kotorcevic, N., Slavkovic, V. & Grujovic, N. (2022). Multi-criteria decision-making methods for selection of lightweight material for railway vehicles. Materials, 16(1), 368. https://doi.org/10.3390/ma16010368
Simon, M. & Joshi, H. (2021). A review on green technologies for the rejuvenation of polluted surface water bodies: Field-scale feasibility, challenges, and future perspectives. Journal of Environmental Chemical Engineering, 9(4), 105763. https://doi.org/10.1016/j.jece.2021.105763
Sinwar, D., Muduli, K., Dhaka, V. S. & Singh, V. (Eds.). (2023). Computational Intelligence Based Optimization of Manufacturing Process for Sustainable Materials. CRC Press.
Tijjani Usman, I. M., Ho, Y. C., Baloo, L., Lam, M. K., Show, P. L. & Sujarwo, W. (2023). Comprehensive review of modification, optimization, and characterisation methods applied to plant-based natural coagulants (PBNCs) for water and wastewater treatment. Sustainability, 15(5), 4484. https://doi.org/10.3390/su15054484
Torrado, A. M., Cortés, S., Salgado, J. M., Max, B., Rodríguez, N., Bibbins, B. P., ... & Domínguez, J. M. (2011). Citric acid production from orange peel wastes by solid-state fermentation. Brazilian Journal of Microbiology, 42, 394-409. https://doi.org/10.1590/S1517-83822011000100049
Villabona-Ortíz, A., Tejada-Tovar, C., Ortega-Toro, R., Licona Dager, N. & Millan Anibal, M. (2023). Natural coagulation as an alternative to raw water treatment. Journal of Water and Land Development, (56). DOI: 10.24425/jwld.2023.143740
Wei, H., Gao, B., Ren, J., Li, A. & Yang, H. (2018). Coagulation/flocculation in dewatering of sludge: A review. Water research, 143, 608-631. https://doi.org/10.1016/j.watres.2018.07.029
Zainol, N. A., Khalilullah, P. A. B., Ghani, A. A., Rashid, N. A. & Makhtar, S. M. Z. (2022). Turbidity Removal from Kaolin Synthetic Wastewater via Coagulation Process Using Sludge from Water Treatment Plant. International Journal of Integrated Engineering, 14(9), 222-231. https://doi.org/10.30880/ijie.2022.14.09.028
Zainol, N. A., Othman, I. S., Zailani, S. N., Ghani, A. A. & Abdullah, S. (2021). Treatment of synthetic turbid water by using natural tamarind seeds. In IOP Conference Series: Earth and Environmental Science (Vol. 765, No. 1, p. 012110). IOP Publishing. 10.1088/1755-1315/765/1/012110
Zhou, L., Han, Y., Li, W. & Zhu, Y. (2021). Study on polymer-bridging flocculation performance of ultrafine specular hematite ore and its high gradient magnetic separation behavior: Description of floc microstructure and flocculation mechanism. Separation and Purification Technology, 276, 119304. https://doi.org/10.1016/j.seppur.2021.11 9304
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